I have managed to get just under 89MPH out of my 1986 90 with a retrofitted Discovery 200TDi and I'm certain it'll do a bit more. I have the standard Defender transfer box but I have 235x85xr16 tyres to help with the gearing (they look good too). I noticed that you said you are getting no smoke - is this even when the engine is under load and / or accelerating up hill? The setup that you have sounds fantastic. An over rated intercooler, paired with an increase in boost will make a world of difference but it sounds to me like you may well be starving the engine of the fuel that it needs for any the extra 'oomph'.
Realistically there should be a whisp of black smoke from the exhaust when you deck the pedal to accelerate away from a stand still, or when you accelerate up hill for example. I'd start by doing as was suggested earlier - give the thing a really good service. New engine, gear box, transfer box and axle oils will make a big difference. Also renew the fuel and air filters to ensure that throughput is optimal. I'd also suggest that you remove the intercooler and throughly swill it out with paraffin or thinners until it runs clean. Allow it to dry and then re-fit.
If that doesn't give you the boost that you were looking for, look into your injection pump fuelling. It may well be that someone has had the boost diaphragm out, and it's very easy for it to have been put back in the wrong position - limiting the amount of fuel that your engine receives under boost.
On the very top of your injection pump you will see four flat head bolts securing a metal cover onto the injection pump housing. Remove the four bolts (they should be very very tight) and then you'll be able to see a circular rubber diaphragm. Push the diaphragm up and down whilst rotating it through a whole 360 degrees in either direction - at the same time also trying to pull it up and out of the recess. Eventually, the diaphragm will lift out of it's recess. There should be:
1x boost diaphragm with attached eccentric boost cone
1x coil spring
1x nylon washer
Put these items to one side and then start the engine. If you look down into the recess, you should see a pin which will have shot all the way across the hole. If it hasn't moved, give the engine a quick blip of full throttle and it should shoot across the hole from right to left (or from the front of the engine towards the back of the engine). If you can't see the pin, it's more than likely ceased, which means that the pump isn't delivering any extra fuel for the increase in turbo boost pressure (your lack of power). If however, the pin has moved out across the hole, turn off the engine and then use a small screw driver to push the pin back towards the front of the engine. Once the pin is al the way back in, pick up the boost diaphragm ready for re-assembly.
When you re-fit the boost diaphragm, you want to position it so that the fuel adjustment pin can travel further out into the hole. The eccentric (off set) cone on the boost diaphragm obviously limits the distance that the fuel adjustment pin can travel out into the hole. In this case, the further the better. So examine the cone and decide which position will allow the pin to extend out its furthest. Push the diaphragm back into it's original position, not forgetting the nylon washer or the coil spring and then re-fit the boost diaphragm lid tightly.
Take it for a spin and then let us know how it goes
Of course, if that doesn't fix the problem, you may have a weak or faulty fuel lift pump (not to be confused with your injection pump), a hole in one of your fuel lines or a split /crack in the boost pressure pipe that runs between the turbo compressor housing and the very top of the injection pump. If this pipe is not connected tight at both ends, or if it has a split, the pressure from the turbo will not push the boost diaphragm down, and you'll get no extra fuel.
-Pos