What do you want to use the vehicle for? Personally I quite like remoulds. Good price and lots of choice of good tread patterns. But if you think it'll be mostly road use, then you might be better off with some new tyres.
In terms of size. 6.00 x 16 are a standard size. About the same as a 205 but narrower. These are not very tall. They can work fine but might not look the best.
7.50 x 16 is a nice size and also a standard fitment. Here are taller tyres. Usually anywhere from 29-31". They are also narrow.
The only trouble is. This is a rare size these days. Michelin XZL's can be had in this size. But are pricey and while tough, not the best performers.
You can still get lots of remoulds in this size. But physical sizes vary a lot. Sadly it's a trend to re-brand 235/85R16's as 7.50's. But a 235 is a fair chunk wider.
On that note. 235/85R16 is a good choice and lots of choice. Technically they are not suitable for standard Series rims as they should be on a 6j rim or wider. And Series are 5.5j wide.
Defender rims can be used, as a 235 is a standard size for Defenders. Or you want to get some after market rims.
With a Series it's a balance of not sticking the tyres out of the arches vs not losing all of your steering lock. Again this depends on you intended use to how important some of these things maybe. And it is possible to add wheel arch extensions or spats.
As for tread patterns. This depends on the use. Aggressive MT's are great off road. But not so on the road. Personally I'd avoid Insa Turbo special tracks unless you really think you need them. I quite like diamonds. And they can be had in 7.50 size.
Terrain and where you are in the country might also dictate what is or isn't a good tread pattern for you.